全文获取类型
收费全文 | 464篇 |
免费 | 12篇 |
国内免费 | 1篇 |
专业分类
电工技术 | 26篇 |
综合类 | 1篇 |
化学工业 | 129篇 |
金属工艺 | 27篇 |
机械仪表 | 14篇 |
建筑科学 | 34篇 |
能源动力 | 10篇 |
轻工业 | 29篇 |
水利工程 | 1篇 |
无线电 | 20篇 |
一般工业技术 | 87篇 |
冶金工业 | 23篇 |
原子能技术 | 16篇 |
自动化技术 | 60篇 |
出版年
2024年 | 1篇 |
2023年 | 1篇 |
2022年 | 2篇 |
2021年 | 8篇 |
2020年 | 3篇 |
2019年 | 8篇 |
2018年 | 14篇 |
2017年 | 8篇 |
2016年 | 13篇 |
2015年 | 8篇 |
2014年 | 11篇 |
2013年 | 23篇 |
2012年 | 34篇 |
2011年 | 40篇 |
2010年 | 23篇 |
2009年 | 43篇 |
2008年 | 20篇 |
2007年 | 13篇 |
2006年 | 14篇 |
2005年 | 16篇 |
2004年 | 10篇 |
2003年 | 20篇 |
2002年 | 12篇 |
2001年 | 10篇 |
2000年 | 9篇 |
1999年 | 13篇 |
1998年 | 12篇 |
1997年 | 7篇 |
1996年 | 4篇 |
1995年 | 6篇 |
1994年 | 14篇 |
1993年 | 5篇 |
1992年 | 7篇 |
1991年 | 7篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1987年 | 2篇 |
1986年 | 9篇 |
1985年 | 7篇 |
1984年 | 4篇 |
1983年 | 2篇 |
1982年 | 2篇 |
1981年 | 1篇 |
1980年 | 2篇 |
1978年 | 1篇 |
1977年 | 2篇 |
1976年 | 2篇 |
1975年 | 1篇 |
1971年 | 1篇 |
排序方式: 共有477条查询结果,搜索用时 609 毫秒
51.
Hiromasa Tawarayama Etsuko Ishikawa Kenji Yamanaka Katsuhisa Itoh Keiko Okada Hiroshi Aoki Hiroaki Yanagita Yoshihiko Matsuoka Hisayoshi Toratani 《Journal of the American Ceramic Society》2000,83(4):792-796
Praseodymium-doped glasses were prepared in the Ga-Na-S (GNS) system and their optical properties were studied. A single-mode fiber with an attenuation loss of 1.2 dB/m at a wavelength of 1.31 μm was fabricated using an extrusion method, and the amplification characteristics were measured in the bidirectional pumping configuration. We demonstrated a gain coefficient of 0.81 dB/mW at a wavelength of 1.34 μm, which is the highest we have ever reported, and achieved a net gain of 32 dB for a pump power of 90 mW. Highly efficient optical amplification at a wavelength of 1.3 μm was demonstrated in the praseodymium-doped GNS fiber. 相似文献
52.
Tsukasa Murayama Masatoshi Shibuya Yoshihiko Yamamoto 《Advanced Synthesis \u0026amp; Catalysis》2016,358(2):166-171
4‐Aryl‐2(1H)‐quinolones were efficiently synthesized via copper‐catalyzed hydroarylation of (o‐aminophenyl)propiolates with arylboronic acid neopentyl glycol esters. The substrate propiolates were prepared from the corresponding silylalkynes with carbon dioxide by Kondo’s carboxylation method using N,N‐dimethylformamide as a solvent. Hydroarylation was performed in the presence of 3 mol% copper(II) acetate in methanol at 28 °C for 12 h and subsequent deprotection using trifluoromethanesulfonic acid (3.0 equiv.) at 65 °C for 2 h in the same pot to afford the desired 4‐aryl‐2(1H)‐quinolones in 39–89% yields.
53.
54.
Sumio Chono Yoshihiko Tauchi Kazuhiro Morimoto 《Drug development and industrial pharmacy》2013,39(1):125-135
ABSTRACTIn order to confirm the efficacy of liposomes as a drug carrier for atherosclerotic therapy, the influence of particle size on the distribution of liposomes to atherosclerotic lesions in mice was investigated. In brief, liposomes of three different particle sizes (500, 200, and 70 nm) were prepared, and the uptake of liposomes by the macrophages and foam cells in vitro and the biodistributions of liposomes administered intravenously to atherogenic mice in vivo were examined. The uptake by the macrophages and foam cells increased with the increase in particle size. Although the elimination rate from the blood circulation and the hepatic and splenic distribution increased with the increase in particle size in atherogenic mice, the aortic distribution was independent of the particle size. The aortic distribution of 200 nm liposomes was the highest in comparison with the other sizes. Surprisingly, the aortic distribution of liposomes in vivo did not correspond with the uptake by macrophages and foam cells in vitro. These results suggest that there is an optimal size for the distribution of liposomes to atherosclerotic lesions. 相似文献
55.
Yoshihiko Hangai Shota Maruhashi Soichiro Kitahara Osamu Kuwazuru Nobuhiro Yoshikawa 《Metallurgical and Materials Transactions A》2009,40(12):2789-2793
The nondestructive and three-dimensional quantitative evaluation of porosity in aluminum alloy die castings is proposed to
identify whether the predominant cause of pore formation is shrinkage or entrapped gas. The validity of this method of evaluation
was shown by comparing two different regions with different ratios of pores formed by shrinkage and gas. It was shown that
the proposed evaluation can be used as a quantitative indication of porosity. 相似文献
56.
Adsorption equilibrium data in lumped water quality indices obtained for diluted solutions of a peat water and effluents from a wastewater treatment were analyzed using the ideal adsorbed solution theory with the Freundlich equation. The use of the same value for Freundlich exponent 1∕n in the ideal adsorbed solution theory resulted in a straightforward and less computationally demanding expression to describe an overall batch adsorption isotherm. A fictive component approach, assuming a logarithmic normal distribution of Freundlich K and a nonadsorbable fraction, adequately described and predicted the overall isotherms for different initial concentrations of diluted solutions presented as a lumped water quality index. The parameters in the distributed fictive component approach were independently sensitive to each portion of an isotherm curvature. Preferential adsorption of the smaller molecular weight (MW) components was observed by a size-exclusion high-performance liquid chromatography. Two-dimensional distribution analysis of organics in terms of Freundlich K and MW revealed a weak tendency of the adsorptive strength to decrease with the increase of the MW. 相似文献
57.
Based on the present state of the art of the separation technology, recycling of fission-product rare elements (FRE) in the FBR spent fuel is discussed. The rad.-waste fractionation is in accordance with the present society's trend toward zero-emission, and the mean of salt-free method utilizing electrochemistry agrees with the principles of the newly established green chemistry. A catalytic electrolytic extraction method is proposed to separate the target, radioactive but potentially strategic elements, Pd, Ru, Rh, Re (Tc), Te and Se dissolved in the HLLW. It avoids secondary waste arising. This method is particularly feasible for the separation of Pd where cyclic reaction of metal cations such as Pd(II) or Fe(II), acting as promoters or mediators and already contained in HLLW, accelerates the electrochemical deposition of Ru, Rh and Re. Elemental separation not only offers alternative material resources to meet expanding demands for catalysts in Fuel Cell/Soft Energy system but is also the first step for transmutation or other selective strategies for waste management of long-lived fission products (LLFP). 相似文献
58.
In this work we report the effects of single stage zone drawing on the properties of NEW-TPI thermoplastic polyimide homopolymer, and its blends with Amoco's Xydar liquid crystalline polymer. Zone drawing was performed first on homopolymer NEW-TPI films to determine the effect of load weight, heater speed, and drawing temperature on the attainable draw ratio. Degree of crystallinity and chain orientation increase as the draw ratio increases for NEW-TPI. Blends of NEW-TPI/Xydar compositions 90/10 and 70/30 were studied next. In blends, the Xydar component is not molecularly dispersed, and is initially preferentially oriented along the machine direction during the film processing stage. Xydar acts as a nucleation site and lowers the temperature for crystallization of the NEW-TPI from the rubbery amorphous state. Zone drawing was performed either parallel or perpendicular to Xydar's initial preferred orientation direction. Blends with lower Xydar fraction could be zone-drawn to higher ratios. Zone drawing perpendicular to Xydar's initial orientation direction also resulted in increased draw ratio. Dynamic mechanical properties of the zone drawn materials were studied. In homopolymer NEW-TPI, dynamic modulus increased by a factor of two to 4.0 GPa in zone drawn films, largely as a result of the formation of oriented crystallites. In the blends, the modulus parallel to Xydar's initial orientation direction was greater than that in the transverse direction. Depending upon composition and test direction, zone drawing increased the dynamic moduli of the blends from 1.5 up to 2.7 times, in the temperature range from 150°C to 300°C. 相似文献
59.
60.
Synthesis of non-equilibrium phases in immiscible metals mechanically mixed by high pressure torsion
Tatsuya Miyazaki Daisuke Terada Yoji Miyajima Challapalli Suryanarayana Reiko Murao Yoshihiko Yokoyama Kazumasa Sugiyama Minoru Umemoto Yoshikazu Todaka Nobuhiro Tsuji 《Journal of Materials Science》2011,46(12):4296-4301
The structural changes in mechanically mixed metals of immiscible combinations of elements caused by bulk mechanical alloying
(MA) through the use of high pressure torsion (HPT) were investigated in Ag–Ni and Nb–Zr systems. There was no alloying between
Ag and Ni on atomic scale even after 100 rotations of HPT. On the other hand, the β-Zr phase started to appear after HPT 2
rotations in the Nb–Zr system, even though β-Zr is a high temperature phase. Further, Nb and Zr were completely mixed to form
a bcc structured single phase after HPT 100 rotations. The sequence of alloying in the Nb–Zr system during HPT was discussed.
These results clearly suggest that non-equilibrium phases can form in the Nb–Zr system by bulk MA by the use of HPT. 相似文献